Rationally Designed Chiral Synthons Enabling Asymmetric Z- and E‑Selective Vinylogous Aldol
Reactions of Aldehydes
Posted on 2018-02-22 - 16:54
In
a conceptually different approach, highly stereoselective 2-oxonia-Cope rearrangement reactions between rationally designed
nonracemic vinylogous aldolation synthons and aldehydes are described
to provide δ-hydroxy-α,β-unsaturated esters with
excellent enantioselectivities and, for the first time, unprecedented Z- and E-selectivities without the regioselectivity
issue.
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Padarti, Akhil; Han, Hyunsoo (2018). Rationally Designed Chiral Synthons Enabling Asymmetric Z- and E‑Selective Vinylogous Aldol
Reactions of Aldehydes. ACS Publications. Collection. https://doi.org/10.1021/acs.orglett.8b00230
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