One-Step Synthesis of Acidophilic
Highly-Photoluminescent
Carbon Dots Modified by Ionic Liquid from Polyethylene Glycol
Posted on 2017-08-31 - 12:13
Acidophilic highly-photoluminescent
ionic liquid (IL)-modified
carbon dots (CDs) were fabricated directly from polyethylene glycol-2000
(PEG2000N) by a simple one-step hydrothermal method in
a system containing an IL (1-butyl-3-methylimidazolium bromide [C4mim]Br) and hydrochloric acid (HCl). In this process, PEG2000N works as the carbon source, [C4mim]Br as the
modifier, and HCl as the accelerator. CDs with low photoluminescence
(PL) intensity and quantum yields (QYs) were generated in the system
without H+, but CDs with high PL intensity and QYs could
be prepared after H+ was introduced. Moreover, with the
increase of H+ concentration, the QYs of the prepared CDs
increase subsequently, and the highest QY reaches up to 43%. The formation
mechanism was explored, and the results showed that H+ changes
the surface groups of the CDs generated without H+ into
those that exist on the CDs generated with H+, which further
improves the PL performance of the CDs. Different from most CDs reported
in the literature, the as-prepared CDs can still exhibit high PL intensity
even under strong acidic condition.
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Chen, Yujuan; Yang, Qian; Xu, Panpan; Sun, Li; Sun, Dong; Zhuo, Kelei (2017). One-Step Synthesis of Acidophilic
Highly-Photoluminescent
Carbon Dots Modified by Ionic Liquid from Polyethylene Glycol. ACS Publications. Collection. https://doi.org/10.1021/acsomega.7b01014
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AUTHORS (6)
YC
Yujuan Chen
QY
Qian Yang
PX
Panpan Xu
LS
Li Sun
DS
Dong Sun
KZ
Kelei Zhuo