Formal [1 + 2 + 3] Annulation: Domino Access to Carbazoles and Indolocarbazole
Alkaloids
Posted on 2018-08-15 - 20:50
A new
formal [1 + 2 + 3] annulation of o-alkenyl
arylisocyanides with α, β-unsaturated ketones under metal-,
base-, and acid-free conditions is disclosed. This domino reaction
provides a general protocol for the efficient and practical synthesis
of a wide range of carbazole derivatives from readily available starting
materials in a single operation. Furthermore, this methodology was
used as the key step in a protecting-group-free synthesis of indolocarbazole
alkaloids arcyriaflavin A and racemosin B.
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Men, Yang; Hu, Zhongyan; Dong, Jinhuan; Xu, Xianxiu; Tang, Bo (2018). Formal [1 + 2 + 3] Annulation: Domino Access to Carbazoles and Indolocarbazole
Alkaloids. ACS Publications. Collection. https://doi.org/10.1021/acs.orglett.8b02266
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AUTHORS (5)
YM
Yang Men
ZH
Zhongyan Hu
JD
Jinhuan Dong
XX
Xianxiu Xu
BT
Bo Tang