A Cascade Dehydrogenative Cross-Coupling/Annulation
Reaction of Benzamides with β‑Keto Esters for the Synthesis
of Isoquinolinone Derivatives
Posted on 2017-11-18 - 15:13
A novel cascade DCC/annulation
reaction of N-alkoxybenzamides
with β-keto esters has been developed for the synthesis of isoquinolinone
derivatives under palladium catalysis. A plausible mechanism involving
α-C(sp2)–H activation and a Pd(II)/Pd(IV)
catalytic cycle is also proposed.
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Xu, Guo-Dong; Huang, Zhi-Zhen (2017). A Cascade Dehydrogenative Cross-Coupling/Annulation
Reaction of Benzamides with β‑Keto Esters for the Synthesis
of Isoquinolinone Derivatives. ACS Publications. Collection. https://doi.org/10.1021/acs.orglett.7b02978
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