Radiochemical Determination of Long-Lived Radionuclides in Proton-Irradiated Heavy Metal Targets: Part II Tungsten

In this study, proton-irradiated tungsten targets, up to 2.6 GeV, were investigated for the purpose of the experimental cross-section measurements. Radiochemical separation methods were applied to isolate the residual long-lived alpha-emitters ¹⁴⁸Gd, ¹⁵⁴Dy, and ¹⁴⁶Sm and the beta-emitters ¹²⁹I and ³⁶Cl from proton-irradiated tungsten targets. The molecular plating technique has been applied to prepare ¹⁴⁸Gd, ¹⁵⁴Dy, and ¹⁴⁶Sm samples for alpha-spectrometry. Production cross-sections of ¹²⁹I and ³⁶Cl were determined by means of accelerator mass spectrometry. The results are compared with theoretical predictions, obtained with the INCL++–ABLA07 codes, showing good agreement for ³⁶Cl and ¹⁴⁸Gd, while a factor of 4 difference was observed for ¹⁵⁴Dy, similar to the results obtained for tantalum targets.