la8b02477_si_001.pdf (3.29 MB)
Solvent-Assisted Tuning of the Size and Shape of CsPbBr3 Nanocrystals via Redispersion Process at Ambient Condition
journal contribution
posted on 2018-11-25, 00:00 authored by Ramavath Babu, Surya Prakash SinghAll-inorganic CsPbBr3 perovskite nanocrystals are emerging
as a new class of semiconductors with outstanding optoelectronic properties
and great potential for various applications, such as, lasing, photon
detection, photovoltaics, etc. This article provides the effect of
solvents on the reprecipitation of CsPbBr3 perovskite at
room temperature. The results observed for CsPbBr3 perovskite
in various antisolvents showed various cubes (nano- to microsized),
self-assembly of nanocubes and nanorods. In addition, all of the various sizes (nano to micro) of cubes and self-assembly of
nanocubes and shape-controlled nanorods exhibited band gap tuning
at the green light region. The corresponding microscopy (field emission
scanning electron microscopy and high-resolution transmission electron
microscopy) images and photoluminescence quantum yield as well as
lifetime decay are presented. To the best of our literature knowledge,
this is the first report on various solvent-assisted studies on CsPbBr3 perovskite nanocrystals.
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Redispersion Processfield emission scanning electron microscopySolvent-Assisted TuningCsPbBr 3 Nanocrystalsnanocubephotoluminescence quantumband gaplight regiontransmission electron microscopyself-assemblyCsPbBr 3 perovskite nanocrystalssolvent-assisted studiesliterature knowledgecubeCsPbBr 3 perovskitephoton detectionAmbient Condition All-inorganic CsPbBr 3 perovskite nanocrystalsroom temperatureshape-controlled nanorodsoptoelectronic propertieslifetime decay
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