ac5b04370_si_001.pdf (152.27 kB)
Remeasurement of 234U Half-Life
journal contribution
posted on 2016-01-29, 00:00 authored by Zsolt Varga, Adrian Nicholl, Maria Wallenius, Klaus MayerThe
half-life of 234U has been measured using a novel
approach. In this method, a uranium material was chemically purified
from its thorium decay product at a well-known time. The ingrowth
of the 230Th daughter product in the material was followed
by measuring the accumulated 230Th daughter product relative
to its parent 234U nuclide using inductively coupled plasma
mass spectrometry. Then, the 234U decay constant and the
respective half-life could be calculated using the radioactive decay
equations based on the n(230Th)/n(234U) amount ratio. The obtained 234U half-life is 244 900 ± 670 years (k = 1), which is in good agreement with the previously reported results
in the literature with comparable uncertainty. The main advantages
of the proposed method are that it does not require the assumption
of secular equilibrium between 234U and 238U.
Moreover, the calculation is independent from the 238U
half-life value and its uncertainty. The suggested methodology can
also be applied for the remeasurement of the half-lives of several
other long-lived radionuclides.