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Programmable Hierarchical Three-Component 2D Assembly at a Liquid−Solid Interface: Recognition, Selection, and Transformation
journal contribution
posted on 2008-08-13, 00:00 authored by Shengbin Lei, Mathieu Surin, Kazukuni Tahara, Jinne Adisoejoso, Roberto Lazzaroni, Yoshito Tobe, Steven De FeyterRecognition and selection are of fundamental importance for the hierarchical assembly of supramolecular systems. Coronene induces the formation of a hydrogen-bonded isophthalic acid supramolecular macrocycle, and this well-defined heterocluster forces, in its turn, DBA1 to form a van der Waals stabilized honeycomb lattice, leading to a three-component 2D crystal containing nine molecules in the unit cell. The recognition and selection events enable efficient error correction and healing in redundant mixtures.
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Transformation Recognitionunit cellDBA 1three-component 2 D crystalerror correctionProgrammable Hierarchical Three-Component 2 D Assemblyvan der WaalsrecognitionInterfacehoneycomb latticemixtureassemblyimportanceselection eventsmoleculeheterocluster forceshealingCoronenesupramolecular systemshydrogen-bonded isophthalic acid supramolecular macrocycle
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