Unveiling the Nontrivial Electronic Structures and
Fermi Topology of High-Temperature Kagome Ferrimagnet HoMn6Sn6
Version 2 2024-12-03, 15:06Version 2 2024-12-03, 15:06
Version 1 2024-11-29, 22:03Version 1 2024-11-29, 22:03
Posted on 2024-12-03 - 15:06
High-temperature
(HT) kagome magnets provide important platforms
to explore nontrivial topological physics and promising potentials
for spintronic applications, due to the complicated interactions among
their electrons, lattices, and magnetism. Herein, the nontrivial electronic
properties of a HT layered kagome-magnet, HoMn6Sn6, are systematically resolved by quantum oscillation measurements
and density functional theory (DFT) calculations. The prominent Shubnikov–de
Haas (SdH) oscillations under pulsed high magnetic fields reveal a
high quantum mobility of 0.37 m2·V–1·s–1 for this HT ferrimagnet. The observed
multiple-frequency quantum oscillations exhibit various angular dependences,
consistent with DFT calculations which suggest a complex Fermi topology
of three three-dimensional hole pockets and two electron pockets.
The observed π shift of the Berry phase for quantum oscillations
unveils nontrivial topological properties in HoMn6Sn6, further confirmed by DFT calculated Dirac fermions and large
anomalous Hall conductivity. Our findings establish HoMn6Sn6 as an HT magnetic candidate for topological magnetoelectronics
or spin quantum applications.
CITE THIS COLLECTION
DataCite
DataCiteDataCite
No result found
Wang, Bin; Huang, Xiang-Fan; Wu, Detong; Zuo, Huakun; Wang, Meng; Hou, Yusheng; et al. (2024). Unveiling the Nontrivial Electronic Structures and
Fermi Topology of High-Temperature Kagome Ferrimagnet HoMn6Sn6. ACS Publications. Collection. https://doi.org/10.1021/acs.nanolett.4c04411