Synthesis and Properties of Quinoidal Fluorenofluorenes
Posted on 2017-09-13 - 14:16
The synthesis and
optoelectronic properties of 24 π-electron,
formally antiaromatic fluoreno[3,2-b]fluorene and
fluoreno[4,3-c]fluorene (FF), are presented. The
solid-state structure of [4,3-c]FF along with computationally
analogous molecules shows that the outer rings are aromatic while
the central four rings possess a bond-localized 2,6-naphthoquinodimethane
motif. The antiaromaticity and biradical character of the FFs is assessed
computationally, the results of which indicate the dominance of the
closed-shell ground state for these molecules.
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Barker, Joshua
E.; Frederickson, Conerd K.; Jones, Michael H.; Zakharov, Lev N.; Haley, Michael M. (2017). Synthesis and Properties of Quinoidal Fluorenofluorenes. ACS Publications. Collection. https://doi.org/10.1021/acs.orglett.7b02605
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AUTHORS (5)
JB
Joshua
E. Barker
CF
Conerd K. Frederickson
MJ
Michael H. Jones
LZ
Lev N. Zakharov
MH
Michael M. Haley