Rapid Access to a Broad Range of 6′-Substituted
Firefly Luciferin Analogues Reveals Surprising Emitters and Inhibitors
Version 3 2017-10-17, 19:04
Version 2 2017-10-17, 16:34
Version 1 2017-10-16, 21:03
Posted on 2017-10-17 - 19:04
Light-emitting firefly
luciferin analogues contain electron-donating
groups in the 6′-position, but the scope of known 6′-substitution
remains narrow. A two-step route to a broad range of 6′-substituted
luciferin analogues was developed to fill this void and enable more
extensive study of the 6′-functionality. This chemistry allowed
direct access to “caged” amide and bright azetidine
analogues, but also revealed thioether inhibitors and unexpectedly
luminogenic aryl amine derivatives.
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Sharma, Deepak
K.; Adams, Spencer T.; Liebmann, Kate L.; Miller, Stephen C. (2017). Rapid Access to a Broad Range of 6′-Substituted
Firefly Luciferin Analogues Reveals Surprising Emitters and Inhibitors. ACS Publications. Collection. https://doi.org/10.1021/acs.orglett.7b02806
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AUTHORS (4)
DS
Deepak
K. Sharma
SA
Spencer T. Adams
KL
Kate L. Liebmann
SM
Stephen C. Miller