Palladium/Lewis Acid Co-catalyzed Divergent Asymmetric
Ring-Opening Reactions of Azabenzonorbornadienes with Alcohols
Version 2 2016-10-03, 15:28
Version 1 2016-09-28, 16:07
Posted on 2016-09-28 - 00:00
By fine tuning the
combinations of chiral palladium catalysts and
Lewis acids, both the additional and reductive asymmetric ring-opening
reactions of azabenzonorbornadienes with alcohols were accomplished
with good chemoselectivity, regioselectivity, and enantioselectivity.
It was proven that the reductive ring-opening products were generated
through a transfer-hydrogenation process with alcohols as hydrogen
source.
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Yang, Fan; Chen, Jingchao; Xu, Jianbin; Ma, Fujie; Zhou, Yongyun; Shinde, Madhuri Vikas; et al. (2016). Palladium/Lewis Acid Co-catalyzed Divergent Asymmetric
Ring-Opening Reactions of Azabenzonorbornadienes with Alcohols. ACS Publications. Collection. https://doi.org/10.1021/acs.orglett.6b02300
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AUTHORS (7)
FY
Fan Yang
JC
Jingchao Chen
JX
Jianbin Xu
FM
Fujie Ma
YZ
Yongyun Zhou
MS
Madhuri Vikas Shinde
BF
Baomin Fan