Nanocross: A Highly Tunable Plasmonic System
Posted on 2017-07-21 - 18:23
With
the help of electron energy loss spectroscopy (EELS) in a scanning
transmission electron microscope (STEM) and boundary element method
(BEM) simulations, we have shown that silver nanocross can be used
to tune the plasmon modes and especially the higher order modes in
a very controlled manner. Morphing a nanorod to a nanocross by growing
another arm along the perpendicular bisector of a nanorod can lead
to a spectacular evolution of various order modes in the EEL spectra.
One can keep a mode fixed in energy while bringing the next higher
order mode close to it, or even make it cross. This allows one to
control the relative separation of energy of the plasmon modes. Hybridization
of individual nanocross plasmon modes have also been studied by bringing
two nanocrosses close together along one of their arms. An analytical
approach based on first order perturbation theory and symmetry arguments
based on group theory aptly fits the experimental observations.
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Das, Pabitra; Lourenço-Martins, Hugo; Tizei, Luiz Henrique Galvão; Weil, Raphaël; Kociak, Mathieu (2017). Nanocross: A Highly Tunable Plasmonic System. ACS Publications. Collection. https://doi.org/10.1021/acs.jpcc.7b05548
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AUTHORS (5)
PD
Pabitra Das
HL
Hugo Lourenço-Martins
LT
Luiz Henrique Galvão Tizei
RW
Raphaël Weil
MK
Mathieu Kociak