Interpretation on Nanoporous Network Structure in
Rice Husk Silica Layer: A Graph Model
Version 2 2018-09-20, 18:51
Version 1 2018-09-20, 18:49
Posted on 2018-09-20 - 18:51
The rice plant produces an amorphous
silica layer in the husk covering
the brown rice grain as a part of a protective respiration system.
The layer shows high permeation molecular flow while the Brunauer–Emmett–Teller
isotherm indicates the existence of nanometer-sized pores. Here, we
interpret the inner structure of the layer as a porous network consisting
of void spheres with a degree of 2–5 and tunnels with a length
of 2–7 nm based on the transmission electron microscopy images.
In the network, the gas molecules travel through the tunnels and move
in random directions after collisions with the walls of the spheres.
A tree network was introduced to understand the permeance of the layer
and the reflection of the molecule of the root or parent sphere was
estimated for a specific case. The tree becomes a graph with cycles
in a finite space such as the silica layer and the reflection of the
root sphere in the graph converses to that of the tree. On the basis
of the properties of the network, the high permeance of the silica
layer in the rice husk can be explained. It is suggested that the
specific system restricts the movements of the gas molecules and can
be applied to reduce the size of gas phase separation and chemical
reactor systems providing a new view to understand nanoscaled porous
materials.
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Lee, Won Jun; Bernasek, Steven L.; Han, Chong Soo (2018). Interpretation on Nanoporous Network Structure in
Rice Husk Silica Layer: A Graph Model. ACS Publications. Collection. https://doi.org/10.1021/acsomega.8b01453
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AUTHORS (3)
WL
Won Jun Lee
SB
Steven L. Bernasek
CH
Chong Soo Han