Hypervalent Iodine-Mediated
Oxidative Rearrangement
of N–H Ketimines: An Umpolung Approach to Amides
Version 2 2017-07-24, 12:12
Version 1 2017-07-24, 11:53
Posted on 2017-07-24 - 12:12
An
umpolung approach to amides via hypervalent iodine-mediated
oxidative rearrangement of N–H ketimines under mild reaction
conditions is described. This strategy provides target amides with
excellent selectivity in good yields. In addition, preliminary mechanistic
studies demonstrated that the migration preference depends on both
steric and electronic effects of the migrating groups.
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Zhao, Zhenguang; Peng, Zhiyuan; Zhao, Yongli; Liu, Hao; Li, Chongnan; Zhao, Junfeng (2017). Hypervalent Iodine-Mediated
Oxidative Rearrangement
of N–H Ketimines: An Umpolung Approach to Amides. ACS Publications. Collection. https://doi.org/10.1021/acs.joc.7b01468
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AUTHORS (6)
ZZ
Zhenguang Zhao
ZP
Zhiyuan Peng
YZ
Yongli Zhao
HL
Hao Liu
CL
Chongnan Li
JZ
Junfeng Zhao