Frequency‑, Time‑, and Wavevector-Resolved
Ultrafast Incoherent Diffraction of Noisy X‑ray Pulses
Posted on 2019-09-18 - 21:14
We
study theoretically incoherent time-resolved X-ray diffraction
of fluctuating sources such as free electron lasers, as well as coherent
sources with controllably added randomness. We find that the temporal
resolution is strongly eroded by the noise. By considering frequency
resolution of the signal, we find that the statistical properties
of the noise carry important information allowing us to restore the
temporal resolution. We propose a multidimensional stochastic resonance
treatment to shape the optical window and extract this information
from signals. Using the frequency-dependent stochastic phase as a
frequency marker allows to improve the spectral resolution as well
via intensity correlations. Frequency-tuned field correlation functions
are used to modify the effective frequency gating and extract specific
charge density contributions to the diffraction pattern while maintaining
temporal resolution.
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Asban, Shahaf; Cho, Daeheum; Mukamel, Shaul (2019). Frequency‑, Time‑, and Wavevector-Resolved
Ultrafast Incoherent Diffraction of Noisy X‑ray Pulses. ACS Publications. Collection. https://doi.org/10.1021/acs.jpclett.9b00924
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AUTHORS (3)
SA
Shahaf Asban
DC
Daeheum Cho
SM
Shaul Mukamel
KEYWORDS
frequency resolutionFrequency-tuned field correlation functionsinformationsourcefrequency gatingelectron lasersWavevector-Resolved Ultrafast Incoherent Diffractiontime-resolved X-ray diffractionfrequency markercharge density contributionsintensity correlationsresonance treatmentdiffraction patternsignal