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Download fileRapid Increase in China’s Industrial Ammonia Emissions: Evidence from Unit-Based Mapping
journal contribution
posted on 2022-02-02, 16:18 authored by Yuang Chen, Qianru Zhang, Xingrui Cai, Haoran Zhang, Huiming Lin, Chaoyue Zheng, Zhanqiang Guo, Shanying Hu, Long Chen, Shu Tao, Maodian Liu, Xuejun WangAmmonia (NH3) is an important
precursor of secondary
inorganic aerosols and greatly impacts nitrogen deposition and acid
rain. Previous studies have mainly focused on the agricultural NH3 emissions, while recent research has noted that industrial
sources could be significant in China. However, detailed estimates
of NH3 emitted from industrial sectors in China are lacking.
Here, we established an unprecedented high-spatial-resolution data
set of China’s industrial NH3 emissions using up-to-date
measurements of NH3 and point source-level information
covering eight major industries and 27 subdivided process categories.
We found that China emitted 798 (90% confidence interval: 668–933)
gigagrams of industrial NH3 into the atmosphere in 2019,
equivalent to 44 ± 20% of the industrial emissions worldwide;
this flux is 3-fold larger than that in 1998 and has fluctuated since
2014. Furthermore, although fertilizer production is responsible for
approximately half of the emissions in China, the emissions from cement
production and coal-fired power plants increased dramatically from
near zero to 164 and 41 gigagrams, respectively, in the past two decades,
primarily due to the NH3 escape caused by the large-scale
application of the denitration process. Our results reveal that, unlike
other major air pollutants, China’s industrial NH3 emission control is still in a critical period, and stricter NH3 emission standards and innovation in pollution control technologies
are highly desirable.
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secondary inorganic aerosolsresolution data setpast two decadesmajor air pollutantsfluctuated since 2014based mapping ammonia668 – 93344 ± 20industrial sources couldpollution control technologiesalthough fertilizer productionindustrial emissions worldwideindustrial ammonia emissionschina emitted 7983 </ subindustrial sectorsemission controlcement productionindustrial nhemissions usingunprecedented highscale applicationresults revealrecent researchrapid increaseprimarily dueprevious studiespoint sourcenear zeromainly focusedimportant precursorhighly desirablefold largerescape causedemission standardsdetailed estimatesdenitration processdate measurementscritical periodconfidence intervalchina ’approximately halfacid rain