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Kinetic Control of Perovskite Thin-Film Morphology and Application in Printable Light-Emitting Diodes
journal contribution
posted on 2017-01-13, 00:00 authored by Prashant Kumar, Baodan Zhao, Richard H. Friend, Aditya Sadhanala, K.S. NarayanHighly
luminescent methylammonium lead bromide (CH3NH3PbBr3) perovskite fibrous microstructure thin films
have been fabricated using a perylene-3,4,9,10-tetracarboxylic dianhydride-containing
antisolvent-mediated single-step fabrication method. Confocal microscopy
of these thin films reveals homogeneous emission over the entire area,
in contrast to the localized emission from the thin films fabricated
by conventional methods. The antisolvent treatment produces pinhole-free,
mazelike morphology with high photoluminescence yield. These films
were incorporated as the emissive layer in thin-film light emitting
diodes (LEDs), made using a low-temperature meltable and processable
alloy as cathode. These LEDs gave luminescence efficiency of up to
50 Cd/m2. The proposed LED structure highlights the prospects
of using low-temperature roll-to-roll processing for manufacturing
perovskite-based solar cells and LEDs.
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Kinetic Controlantisolvent treatmentluminescence efficiencyemissive layerPerovskite Thin-Film MorphologyCH 3 NH 3 PbBr 3Confocal microscopyemissionmanufacturing perovskite-basedroll-to-roll processingmazelike morphologyLED structureprocessable alloyPrintable Light-Emitting Diodesfabrication methodthin-film light
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