10.1021/acs.chemmater.8b00945.s004
Jiang Wu
Jiang
Wu
Fengjun Ye
Fengjun
Ye
Wenqiang Yang
Wenqiang
Yang
Zhaojian Xu
Zhaojian
Xu
Deying Luo
Deying
Luo
Rui Su
Rui
Su
Yifei Zhang
Yifei
Zhang
Rui Zhu
Rui
Zhu
Qihuang Gong
Qihuang
Gong
Perovskite Single-Crystal Microarrays for Efficient
Photovoltaic Devices
American Chemical Society
2018
Perovskite Single-Crystal Microarrays
uniform perovskite single-crystal microarrays
patterning
NH
CH
ORAP process
Efficient Photovoltaic Devices Hybrid perovskite
perovskite single-crystal microarrays
optoelectronic devices
2018-07-11 18:23:36
Media
https://acs.figshare.com/articles/media/Perovskite_Single-Crystal_Microarrays_for_Efficient_Photovoltaic_Devices/6806942
Hybrid perovskite single crystals
offer a great promise for optoelectronic
devices, and patterning is broadly required in industrialized applications
for functional purposes. However, established patterning techniques
meet their limitations when it comes to hybrid perovskite single crystals
with multilayered diode structures. In this work, an Ostwald ripening
assisted photolithography (ORAP) patterning process, which employs
wettability-assisted blade-coating and Ostwald ripening assisted crystallization,
is developed for fabricating patterned perovskite single-crystal microarrays.
Optoelectronic devices based on uniform perovskite single-crystal
microarrays with a multilayered diode structure can be constructed
through the ORAP process. To demonstrate the compatibility of the
ORAP process with the manufacture of optoelectronic devices, patterned
CH<sub>3</sub>NH<sub>3</sub>PbBr<sub>3</sub> single-crystal
microarray solar cells, which show enhanced performance than solar
cells based on CH<sub>3</sub>NH<sub>3</sub>PbBr<sub>3</sub> continuous
single crystals reported, were fabricated. With the development of
perovskite research, we are confident that the ORAP process opens
a new avenue to fabricate optoelectronic devices based on perovskite
microarrays.