Kimberg, Victor Bin Zhang, Song Rohringer, Nina The number of AXE photons emitted at different lasing transitions (a) and the AXE spectrum on the C 1s<sup>−1</sup> → <em>X</em> transition as a function of the interaction length (b) <p><strong>Figure 5.</strong> The number of AXE photons emitted at different lasing transitions (a) and the AXE spectrum on the C 1s<sup>−1</sup> → <em>X</em> transition as a function of the interaction length (b). (c) Fluorescence (−− − −) and AXE (\full) spectra on the C 1s<sup>−1</sup> → <em>X</em> (1), O 1s<sup>−1</sup> → <em>A</em> (2) and O 1s<sup>−1</sup> → <em>B</em> (3) transitions at the end of the medium at <em>z</em> = 5 mm. All simulations are done for an isotropic molecular ensemble, and for an XFEL pump pulse of duration 50 fs containing 3.6 <b>×</b> 10<sup>12</sup> photons.</p> <p><strong>Abstract</strong></p> <p>We theoretically demonstrate the feasibility of x-ray lasing in the CO molecule by the core ionization of the C K- and O K-shell by x-ray free-electron laser sources. Our numerical simulations are based on the solution of generalized Maxwell–Bloch equations, accounting for the electronic and nuclear degrees of freedom. The amplified x-ray emission pulses have an extremely narrow linewidth of about 0.1 eV and a pulse duration shorter than 30 fs. We compare x-ray lasing transitions to the three lowest electronic states of singly ionized CO. The dependence of the lasing efficiency on the spectral width of the x-ray fluorescence band, value and orientation of the electronic transition dipole moment, lifetime of the core-excited state and the duration of the pump pulse is analysed. Using a pre-aligned molecular ensemble substantially increases the amplified emission. Moreover, by controlling the molecular alignment and thereby the alignment of the transition dipole moment polarization, the control of the emitted x-ray radiation is achievable. Preparing the initial vibrational quantum state, the x-ray emission frequency can be tuned within the fluorescence band. The present scheme is applicable to other diatomic systems, thereby extending the spectral range of coherent x-ray radiation sources based on stimulated x-ray emission on bound transitions.</p> axe;vibrational quantum state;emission;co;lasing;xfel;duration 50 fs;transition;pulse;C 1;Atomic Physics;Molecular Physics 2013-08-13
    https://iop.figshare.com/articles/figure/_The_number_of_AXE_photons_emitted_at_different_lasing_transitions_a_and_the_AXE_spectrum_on_the_C_1/1012420
10.6084/m9.figshare.1012420.v1